5.4.1.2 Catalyst bulk solubility tuning -- 5.4.1.3 Designed solubility by alloying -- 5.4.1.4 Growth on liquid surfaces -- 5.4.1.5 Solid source precursors -- 5.4.2 Transfer routes overview -- 5.4.3 State-of-the-art: large area single 2D crystal production -- 5.4.3.1 Single domain growth -- 5.4.3.2 Domain stitching -- 5.4.3.3 Large area production -- 5.5 Conclusions and outlook -- References -- 6 Realization of electronic-grade two-dimensional transition metal dichalcogenides by thin-film deposition techniques -- 6.1 Current challenges in transition metal dichalcogenide synthesis -- 6.2 Current synthesis techniques -- 6.2.1 Reactor design -- 6.2.2 Solid-source chemical vapor deposition (SS-CVD) -- 6.2.3 Metal-organic chemical vapor deposition (MOCVD) -- 6.2.4 Molecular beam epitaxy (MBE) -- 6.3 Controlling nucleation and crystal growth -- 6.3.1 Substrate engineering -- 6.3.2 Precursor chemistry -- 6.3.3 Impact of growth temperature -- 6.3.4 Impact of growth pressure -- 6.4 Materials engineering -- 6.4.1 Defect engineering -- 6.4.2 Heterostructures -- 6.4.3 Doping and alloying -- 6.5 Summary -- Note -- Acknowledgments -- References -- 7 Materials engineering - defect healing & -- passivation -- 7.1 Introduction -- 7.2 Defect formation and healing in 2D TMDs -- 7.2.1 Point defects -- 7.2.2 Line defects -- 7.3 Defect engineering by chemical treatment and applications -- 7.3.1 Vacancy healing -- 7.3.2 Covalent functionalization -- 7.3.3 Interfacial charge transfer -- 7.4 Defect control by external sources -- 7.4.1 Thermal annealing -- 7.4.2 Electron beam irradiation -- 7.4.3 Plasma treatment -- 7.4.4 Encapsulation -- 7.5 Future perspectives -- References -- 8 Nonequilibrium synthesis and processing approaches to tailor heterogeneity in 2D materials -- 8.1 Introduction.

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